吉林大学学报(地球科学版) ›› 2017, Vol. 47 ›› Issue (3): 868-873.doi: 10.13278/j.cnki.jjuese.201703207
宋志伟, 李婷, 易宏云, 邱杰, 张迪, 陈丹凤
Song Zhiwei, Li Ting, Yi Hongyun, Qiu Jie, Zhang Di, Chen Danfeng
摘要: 为探讨好氧颗粒污泥对有机污染物的吸附机制,采用动态吸附方式研究好氧颗粒污泥对有机污染物的初期吸附作用,采用静态吸附方式考察好氧颗粒污泥失活前后对有机污染物吸附效率的差异,分析了好氧颗粒污泥吸附有机污染物前后的热力学参数及红外光谱变化。结果表明,好氧颗粒污泥对有机污染物的吸附过程表现出了明显的初期吸附去除现象,30 min内对有机污染物吸附去除率达60.19%。好氧颗粒污泥吸附有机污染物是一个自发、吸热、熵增的过程,且吸附过程是一个以物理吸附为主、生物吸附和化学吸附为辅的复杂过程。
中图分类号:
[1] 张自杰,周帆. 活性污泥生物学与反应学动力学[M]. 北京:中国环境科学出版社,1989. Zhang Zijie, Zhou Fan. Activated Sludge Biology and Kinetics [M]. Beijing: Chinese Environment Science Press,1989. [2] 徐宏英,李亚新,苏槟楠,等.厌氧颗粒污泥对有机污染物的初期吸附机制[J].环境科学与技术,2010,33(9):75-78,191. Xu Hongying, Li Yaxin, Su Binnan, et al. Initial Adsorption Mechanism of Anaerobic Granular Sludge to Organic Pollutants [J]. Environmental Science and Technology, 2010, 33(9): 75-78,191. [3] 季民,魏燕杰,李超,等.好氧颗粒污泥处理实际污(废)水的研究与工程化应用进展[J].中国给水排水,2013,26(4):10-14. Ji Min, Wei Yanjie, Li Chao, et al. Research of Treatment of Sewage (Waste) Water by Aerobic Granular Sludge and Progress in Engineering Application [J]. China Water & Wastewater, 2013,26(4):10-14. [4] 熊光城,濮文虹,杨昌柱.预加不同比例不同粒径好氧颗粒对SBR中好氧颗粒污泥形成的影响[J].环境科学,2013,34(4): 1472-1478. Xiong Guangcheng, Pu Wenhong, Yang Changzhu. Effect of Aerobic Granular Sludge Formation in SBR by Adding Aerobic Granule of Different Proportion and Different Particle Size [J]. Environmental Science, 2013,34 (4): 1472-1478. [5] 王昌稳,李军,赵白航,等.好氧颗粒污泥的快速培养与污泥特性分析[J].中南大学学报(自然科学版), 2013, 44(6):2623-2628. Wang Changwen, Li Jun, Zhao Baihang, et al. Rapid Development of Aerobic Granular Sludge and Sludge Characteristics Analysis [J]. Journal of Central South University(Science and Technology), 2013, 44 (6): 2623-2628. [6] 刘国洋,赵白航,李军,等.好氧颗粒污泥降解苯酚[J].环境工程学报, 2014, 8(9):3645-3650. Liu Guoyang, Zhao Baihang, Li Jun, et al. The Degradation of Phenol by Aerobic Granular Sludge [J]. Chinese Journal of Environmental Engineering, 2014, 8 (9): 3645 -3650. [7] Jian M P, Tang C C, Liu M. Adsorptive Removal of Cu2+ from Aqueous Solution Using Aerobic Granular Sludge[J].Desalination and Water Treatment, 2015, 54(7):2005-2014. [8] Ni S Q, Cui Q J, Zheng Z. Interaction of Polybro-minated Diphenyl Ethers and Aerobic Granular Sludge: Biosorption and Microbial Degradation[J/OL]. Biomed Research International,2014.http://dx.doi.org/10.1155/2014/274620. [9] 宋志伟,王秋旭,宁婷婷,等.微生物絮凝剂投加方式对好氧颗粒污泥性能的影响[J]. 吉林大学学报(地球科学版),2015,45(1): 247-254. Song Zhiwei, Wang Qiuxu, Ning Tingting, et al. Effect of Microbial Flocculant on the Performance of Aerobic Granular Sludge [J]. Journal of Jilin University (Earth Science Edition), 2015,45 (1): 247-254. [10] 国家环境保护总局.水和废水监测分析方法[M].4版.北京:中国环境科学出版社,2002. State Environmental Protection Administration. Monitoring Analysis Method Water and Wastewater [M]. 4th Ed. Beijing: China Environmental Science Press, 2002. [11] 倪正.活性污泥胞外聚合物提取条件优化及对Pb2+吸附性能和机理的研究[D].芜湖:安徽工程大学,2012: 3-4. Ni Zheng. Extracellular Polymeric Substances Extraction Condition Optimization and Adsorption of Pb2+ and Mechanism Research of Activated Sludge[D]. Wuhu: Anhui University of Engineering, 2012: 3-4. [12] 毛艳萍,陈泉源,杜菲菲.酸热处理提剩余污泥胞外聚合物的条件优化[J].环境工程学报,2012,6(9) : 3294-3298. Mao Yanping, Chen Quanyuan, Du Feifei. Optimization of the Conditions for the Extraction of Excess Sludge Extracellular Polymeric by Acid Heat Treatment[J]. Chinese Journal of Environmental Engineering, 2012,6 (9): 3294-3298. [13] 李新.活性污泥法理论与技术[M].北京:中国建筑工业出版社,2007:125-127. Li Xin. Theory and Technology of Activated Sludge Process[M]. Beijing: China Building Industry Press, 2007: 125-127. [14] 王建龙,张子健,吴伟伟.好氧颗粒污泥的研究进展[J].环境科学学报,2009,29(3):449-473. Wang Jianlong, Zhang Zijian, Wu Weiwei. Research Progress of Aerobic Granular Sludge [J]. Journal of Environmental Science, 2009,29 (3): 449-473. [15] 蒋礼源,刘绍根,王国明.活性污泥与失活污泥的吸附性能比较[J].工业用水与废水,2007,38(5):42-45. Jiang Liyuan, Liu Shaogen, Wang Guoming. Comparison of the Adsorption Capacity of Living and Non-Living Sludge [J]. Industrial Water and Wastewater, 2007,38 (5): 42-45. [16] Aksu Z, Tezer S. Equilibrium and Kinetic Modelling of Biosorption of Remazol Black B by Rhizopus Arrhizusin a Batch System: Effect of Temperature[J]. Process Biochem, 2000,36(5): 431-439. |
[1] | 游远航. 广州地区蔬菜生产基地有机污染物含量状况及分布[J]. 吉林大学学报(地球科学版), 2015, 45(4): 1205-1216. |
[2] | 宋志伟, 王秋旭, 宁婷婷, 任南琪, 李立欣. 微生物絮凝剂投加方式对好氧颗粒污泥性能的影响[J]. 吉林大学学报(地球科学版), 2015, 45(1): 247-254. |
[3] | 何俊,冶雪艳. 基于有机污染物扩散的复合衬垫厚度的概率设计[J]. 吉林大学学报(地球科学版), 2013, 43(1): 228-234. |
[4] | 董德明, 宋兴, 花修艺, 袁懋, 梁建海, 郭志勇, 梁大鹏. 吉林省典型废水COD与TOC的相关关系及其形成机制和影响因素[J]. J4, 2012, 42(5): 1446-1455. |
[5] | 周丹丹, 刘孟媛, 侯典训, 王紫嫣, 梁爽, 董双石. 连续流气提式流化床启动过程中好氧颗粒污泥的形成机制[J]. J4, 2012, 42(1): 212-219. |
[6] | 宋志伟, 程晓霞, 乔艳云, 潘宇, 罗克洁. 接种污泥对好氧颗粒污泥稳定性的影响[J]. J4, 2011, 41(3): 873-878. |
|