吉林大学学报(理学版) ›› 2021, Vol. 59 ›› Issue (3): 713-718.

• • 上一篇    

TiO2-GO复合材料对苯酚废水的吸附行为

夏爱清, 邢翠娟, 于玲, 郭云飞   

  1. 邢台学院 化学与化工学院, 河北 邢台054001
  • 收稿日期:2020-10-05 出版日期:2021-05-26 发布日期:2021-05-23
  • 通讯作者: 夏爱清 E-mail:xiaaiqing59420@sina.com

Adsorption Behavior of GO-TiO2 Composites on Phenol Wastewater

XIA Aiqing, XING Cuijuan, YU Ling, GUO Yunfei   

  1. School of Chemistry and Chemical Engineering,  Xingtai University, Xingtai 054001,  Hebei Province,  China
  • Received:2020-10-05 Online:2021-05-26 Published:2021-05-23

摘要: 采用一锅超声回流法制备一种新型的二氧化钛-氧化石墨烯(TiO2-GO)复合材料, 通过X射线衍射(XRD)、红外光谱(IR)和 Raman光谱对其结构进行表征, 并研究溶液的pH值、 吸附温度、 吸附时间、 溶液的初始质量浓度对该材料作为吸附剂对苯酚废水去除效果的影响. 实验结果表明: 400 mg/L的苯酚溶液, 室温下, pH=5时,该材料对苯酚的吸附量为80 mg/g;吸附过程符合Langmuir模型,动力学实验数据符合准二级动力学曲线; TiO2-GO可在30 min内有效净化苯酚废水,具有一定的应用前景.

关键词: 二氧化钛-氧化石墨烯, 复合材料, 吸附, 苯酚

Abstract: A new type  of TiO2-graphene oxide (TiO2-GO) composite was prepared by  one-pot ultrasonic reflux method,and its structure was characterized by X-ray diffraction (XRD), infrared spectrum (IR) and Raman spectrum, and  the removal effect of the material as an adsorbent on phenol wastewater was studied at different pH values, adsorption temperature, adsorption time and initial mass concentration of the solution. The experimental results show that when the mass concentration of  phenol solution is 400 mg/L, the adsorption capacity of phenol is 80 mg/g at room temperature with  pH=5. The adsorption process is  in accordance with the Langmuir model, and the kinetic experimental data are in accordance with the quasi-second\|order kinetic curves.  TiO2-GO  can effectively purify phenol wastewater within 30 min, which has a certain  application prospect.

Key words: titanium dioxide-graphene oxide, composite, adsorption, phenol

中图分类号: 

  • X131.2