Journal of Jilin University(Earth Science Edition) ›› 2020, Vol. 50 ›› Issue (2): 368-377.doi: 10.13278/j.cnki.jjuese.20190309

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Response Mechanism Between Oil Yield and Total Organic Carbon of Non-Marine Oil Shale in China

Jia Jianliang1, Liu Zhaojun2, Meng Qingtao2, Sun Pingchang2, Xu Jinjun3, Liu Rong2, Bai Yueyue4   

  1. 1. Institute of Geology, Chinese Academy of Geological Sciences, Beijing 100037, China;
    2. College of Earth Sciences, Jilin University, Changchun 130061, China;
    3. School of Geosciences, China University of Petroleum(East China), Qingdao 266580, China;
    4. SinoProbe Center, Chinese Academy of Geological Sciences, Beijing 100037, China
  • Received:2019-12-25 Online:2020-03-26 Published:2020-03-31
  • Supported by:
    Supported by National Natural Science Foundation of China (41772114, 41402123), Project of China Geological Survey (DD2019005) and Central Public-Interest Scientific Institution Basal Research Fund (JYYWF20180901)

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Abstract: In order to establish the reliable model between oil yield and total organic carbon (TOC) of oil shale to predict oil yield, it is very important to reveal the response mechanism between oil yield and TOC in different genetic types of oil shale of continental basins. In this paper, the response mechanism between oil yield and TOC in non-marine oil shale was studied by using the key parameters of borehole cores in various types of basins combined with sedimentology, organic geochemistry, and thermal simulation. The results show that an excellent correlation (R2=0.81-0.97) between oil yield and TOC exists in oil shales from different types of basins and sedimentary backgrounds. Firstly, the non-marine oil shale is divided into five genetic types, which control the relationship between oil yield and TOC. Secondly, three weight-loss stages of oil shales were presented during heating simulation, which clarifies the specific physical significance of oil yield and TOC parameters. Finally, the oil shale formed in similar basin and sedimentary background has similar organic matter source, so it has roughly equivalent hydrocarbon regeneration efficiency. The genetic types of non-marine oil shale, the physical significance of oil yield and TOC parameters, and the hydrocarbon regeneration capacity of oil shale were used to understand the internal relationship between oil yield and TOC of non-marine oil shale in China.

Key words: continental basin, oil shale, oil yield, total organic carbon, genetic type, thermal simulation, hydrocarbon generation efficiency, response mechanism

CLC Number: 

  • P618.12
[1] 贾建亮, 刘招君, 陈永成. 油页岩的地震识别与评价技术[J]. 中南大学学报(自然科学版), 2015, 46(7):2581-2589. Jia Jianliang, Liu Zhaojun, Chen Yongcheng. A Seismic Technique for Recognition and Evaluation of Oil Shale[J]. Journal of Central South University, 2015, 46(7):2581-2589.
[2] 刘招君, 孟庆涛, 贾建亮. 油页岩成矿作用研究中的关键方法和技术[J]. 古地理学报, 2019, 21(1):133-148. Liu Zhaojun, Meng Qingtao, Jia Jianliang. Key Methods and Technologies in the Study of Oil Shale Mineralization[J]. Journal of Palaeogeography, 2019, 21(1):133-148.
[3] 贺君玲, 邓守伟, 陈文龙, 等. 利用测井技术评价松辽盆地南部油页岩[J]. 吉林大学学报(地球科学版), 2006, 36(6):909-914. He Junling, Deng Shouwei, Chen Wenlong, et al. Evaluation of Oil Shale in the Southern Songliao Basin Using Logging Techniques[J]. Journal of Jilin University (Earth Science Edition), 2006, 36(6):909-914.
[4] Jia J L, Liu Z J, Meng Q T, et al. Quantitative Evaluation of Oil Shale Based on Well Log and 3-D Seismic Technique in the Songliao Basin, NE China[J]. Oil Shale, 2012, 29(2):128-150.
[5] 柳少鹏, 周世新, 王保忠, 等. 烃源岩评价参数与油页岩品质指标内在关系探讨[J]. 天然气地球科学, 2012, 23(3):561-569. Liu Shaopeng, Zhou Shixin, Wang Baozhong, et al. Relationship Between Industrial Indexes and Source Rock Evaluation Parameters of Oil Shale[J]. Natural Gas Geoscience, 2012, 23(3):561-569.
[6] 贾建亮. 基于地球化学-地球物理的松辽盆地上白垩统油页岩识别与资源评价[D]. 长春:吉林大学, 2012. Jia Jiangliang. Research on the Recognition and Resource Evaluation of the Upper Cretaceous Oil Shale Based on Geochemistry-Geophysics Technique in the Songliao Basin, China[D]. Changchun:Jilin University, 2012.
[7] 李宝毅, 王建鹏, 徐银波, 等. 断陷和坳陷盆地富有机质泥岩测试参数及研究意义[J]. 世界地质, 2012, 31(4):778-784. Li Baoyi, Wang Jianpeng, Xu Yinbo, et al.Testing Parameters of Organic-Rich Mudstone in Faulted Basin and Depressed Basin and Their Significance[J]. Global Geology, 2012, 31(4):778-784.
[8] Зеленин Н И, Oзеров N M. Справочник по Горючим Сланцам[M]. Л:Недра, 1983.
[9] 刘招君, 孟庆涛, 柳蓉.中国陆相油页岩特征及成因类型[J]. 古地理学报, 2009, 11(1):105-114. Liu Zhaojun, Meng Qingtao, Liu Rong. Characteristics and Genetic Types of Continental Oil Shales in China[J]. Journal of Palaeogeography, 2009, 11(1):105-114.
[10] Yu Fengning,Sun Pingchang,Zhao Kang'an,et al. Experimental Constraints on the Evolution of Organic Matter in Oil Shales During Heating:Implications for Enhanced in Situ Oil Recovery from Oil Shales[J/OL]. Fuel, (2019-10-02)[2019-12-23] doi:10.1016/j.fuel.2019.116412.
[11] 刘招君, 孙平昌, 柳蓉, 等. 中国陆相盆地油页岩成因类型及矿床特征[J]. 古地理学报, 2016, 18(4):525-534. Liu Zhaojun, Sun Pingchang, Liu Rong, et al. Genetic Types and Deposit Features of Oil Shale in Continental Basin in China[J]. Journal of Palaeogeography, 2016, 18(4):525-534.
[12] Bechtel A, Jia J L, Strobl A I S, et al.Palaeoenvironmental Conditions During Deposition of the Upper Cretaceous Oil Shale Sequences in the Songliao Basin (NE China):Implications from Geochemical Analysis[J]. Organic Geochemistry, 2012, 46:76-95.
[13] Jia J, Liu Z J, Bechtel A, et al. Tectonic and Climate Control of Oil Shale Deposition in the Upper Cretaceous Qingshankou Formation (Songliao Basin, NE China)[J]. International Journal of Earth Sciences, 2013, 102(6):1717-1734.
[14] Jia J, Bechtel A, Liu Z J, et al. Oil Shale Formation in the Upper Cretaceous Nenjiang Formation of the Songliao Basin (NE China):Implications from Organic and Inorganic Geochemical Analyses[J]. International Journal of Coal Geology, 2013, 113(4):11-26.
[15] 贾建亮, 刘招君, Achim B, 等. 松辽盆地嫩江组油页岩发育控制因素[J]. 地球科学:中国地质大学学报, 2014, 39(2):174-186. Jia Jianliang, Liu Zhaojun, Achim B, et al.Major Factors Controlling Formation of Oil Shale in Nenjiang Formation of Songliao Basin[J]. Earth Science:Journal of China University of Geosciences, 2014, 39(2):174-186.
[16] Xu J, Liu Z, Bechtel A, Meng Q T, et al.Basin Evolution and Oil Shale Deposition During Upper Cretaceous in the Songliao Basin (NE China):Implications from Sequence Stratigraphy and Geochemistry[J]. International Journal of Coal Geology, 2015, 149:9-23.
[17] 孙平昌. 松辽盆地东南部上白垩统含油页岩系有机质富集环境动力学[D]. 长春:吉林大学, 2013. Sun Pingchang. Environmental Dynamics of Organic Accumulation in the Oil Shale Bearing Layers in the Upper Cretaceous, Southeast Songliao Basin (NE China)[J]. Changchun:Jilin University, 2013.
[18] 王君贤, 刘招君, 孙平昌, 等. 柴北缘鱼卡地区中侏罗统油页岩类型及成矿差异[J]. 大庆石油地质与开发, 2017, 36(4):168-174. Wang Junxian, Liu Zhaojun, Sun Pingchang, et al. Types and Mineralizing Differences for Middle Jurassic Oil Shale in Yuqia Region of North Margin in Qaidam Basin[J]. Petroleum Geology and Oilfield Development in Daqing, 2017, 36(4):168-174.
[19] Meng Q T, Sun P C, Liu Z, et al. Characteristic and Accumulation of Middle Jurassic Oil Shale in the Yuqia Area, Northern Qaidam Basin, Northwest China[J]. Oil Shale, 2018, 35(1):1-25.
[20] 曾文人, 孟庆涛, 刘招君, 等.柴北缘团鱼山地区中侏罗统石门沟组油页岩有机地球化学特征及古湖泊条件[J]. 吉林大学学报(地球科学版), 2019, 49(5):1270-1284. Zeng Wenren, Meng Qingtao, Liu Zhaojun, et al.Organic Geochemical Characteristics and Paleo-Lake Conditions of Oil Shale of Middle Jurassic Shimengou Formation in Tuanyushan Area of Northern Qaidam Basin[J]. Journal of Jilin University (Earth science edition), 2019, 49(5):1270-1284.
[21] 孙平昌, 刘招君, 孟庆涛, 等. 桦甸盆地古近纪充填特征及对油页岩成矿的影响[J]. 煤炭学报, 2011, 36(7):1110-1116. Sun Pingchang, Liu Zhaojun, Meng Qingtao, et al. Effect of the Basin-Fill Features on Oil Shale Formation in Paleogene, Huadian Basin[J]. Journal of Coal, 2011, 36(7):1110-1116.
[22] 孟庆涛, 刘招君, 胡菲, 等. 桦甸盆地始新世古湖泊生产力与有机质富集机制[J]. 中国石油大学学报(自然科学版), 2012, 36(5):38-44. Meng Qingtao, Liu Zhaojun, Hu Fei, et al.Productivity of Eocene Ancient Lake and Enrichment Mechanism of Organic Matter in Huadian Basin[J]. Journal of China University of Petroleum, 2012, 36(5):38-44.
[23] Sun P C, Sachsenhofer R F, Liu Z J, et al.Organic Matter Accumulation in the Oil Shale-and Coal-Bearing Huadian Basin (Eocene; NE China)[J]. International Journal of Coal Geology, 2013, 105(1):1-15.
[24] Strobl S A I,Sachsenhofer R F, Bechtel A, et al. Deposition of Coal and Oil Shale in NE China:The Eocene Huadian Basin Compared to the Coeval Fushun Basin[J]. Marine and Petroleum Geology, 2015, 64(6):347-362.
[25] 刘招君, 杨虎林, 董清水, 等. 中国油页岩[M]. 北京:石油出版社, 2009. Liu Zhaojun, Yang Hulin, Dong Qingshui, et al. Oil Shale in China[M]. Beijing:Petroleum Industry Press, 2009.
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