吉林大学学报(地球科学版) ›› 2018, Vol. 48 ›› Issue (5): 1451-1464.doi: 10.13278/j.cnki.jjuese.20170087

• 地质工程与环境工程 • 上一篇    下一篇

陕西省泾惠渠灌区地下水污染与人体健康风险评价

张艳1,2, 徐斌3,4, 刘秀花3,4   

  1. 1. 长安大学地球科学与资源学院, 西安 710054;
    2. 陕西省土地整治重点实验室, 西安 710054;
    3. 长安大学环境科学与工程学院, 西安 710054;
    4. 旱区地下水文与生态效应教育部重点实验室(长安大学), 西安 710054
  • 收稿日期:2017-12-28 发布日期:2018-11-20
  • 作者简介:张艳(1978-),女,副教授,博士,主要从事地理信息系统、环境生态安全方面的研究,E-mail:zyzhangy@chd.edu.cn
  • 基金资助:
    国家自然科学基金项目(41273104);高等学校学科创新引智计划(B08039);陕西省土地整治重点实验室开放基金(2018-JC09)

Groundwater Contamination and Human Health Risk Assessment in Jinghui Irrigation District, Shaanxi Province

Zhang Yan1,2, Xu Bin3,4, Liu Xiuhua3,4   

  1. 1. School of Earth Science and Resources, Chang'an University, Xi'an 710054, China;
    2. Shaanxi Key Laboratory of Land Consolidation, Xi'an 710054, China;
    3. School of Environmental Science and Engineering, Chang'an University, Xi'an 710054, China;
    4. Key Laboratory of Subsurface Hydrology and Ecological Effects in Arid Region(Chang'an University), Ministry of Education, Xi'an 710054, China
  • Received:2017-12-28 Published:2018-11-20
  • Supported by:
    Supported by National Science Foundation of China (41273104), Subjects Innovation and Talents Introduction Plan of Colleges and Universities (B08039) and Fund Project of Shaanxi Key Laboratory of Land Consolidation(2018-JC09)

摘要: 为了研究陕西省泾惠渠灌区地下水污染特征及人体健康风险状况,采集地下水样品进行分析测定,首先运用单因子指数法进行污染评价,再利用GIS获取主要污染物As、Cr (Ⅵ)和NO3--N的空间分布特征,最后借鉴美国环境保护署的人体健康风险评价模型对灌区地下水污染物的人体健康风险做出评价。结果表明:研究区地下水中As、Cr (Ⅵ)、NO3--N的质量浓度均超标,As对成人的致癌风险最高达3.50×10-4,明显超出限值1.00×10-4,长期暴露对当地居民带来罹患癌症的健康风险较高;As、Cr (Ⅵ)、NO3--N的非致癌风险从大到小排序为Cr (Ⅵ)、NO3--N、As,其中Cr (Ⅵ)对儿童的非致癌风险最高,达8.693 7,远超限值1.000 0,危害性最大。空间分布特征方面,As的致癌风险区域面积比例最高,为42.82%,As、Cr (Ⅵ)、NO3--N的非致癌风险区域面积比例分别高达69.19%、69.06%和66.55%,水安全问题突出。

关键词: 地下水, 污染, 人体健康, 风险评价, 泾惠渠灌区

Abstract: In order to investigate the potential human health risk of groundwater contamination in the Jinghui irrigation district in Shaanxi Province, the samples of groundwater were collected, and their physical and chemical characteristics were analyzed through laboratory test. The contamination was evaluated by using a single factor index method, and the spatial distribution of As, Cr(Ⅵ) and NO3--N were obtained by GIS. The human health risk of the groundwater contaminants were assessed by using human health risk assessment model. The results show that the concentration of As, Cr(Ⅵ) and NO3--N of groundwater in the study area exceeds the limits, the carcinogenic risk of As for adults reaches 3.50×10-4, beyond the limit of 1.00×10-4. A long-term exposure to As increases the risk of getting cancer. The ranking of non-carcinogenic risk of As, Cr(Ⅵ) and NO3--N is Cr(Ⅵ) > NO3--N > As,the non-carcinogenic risk of Cr(Ⅵ) for children reaches 8.693 7, far beyond the limit of 1.000 0. The human health risks resulted from oral exposure to the three contaminants are higher than those from dermal exposure. Spatially, As carcinogenic risk area is up to 42.82%, and the area ratios of the non-carcinogenic risk caused by As, Cr(Ⅵ) and NO3--N are 69.19%、69.06% and 66.55% respectively, the local water safety is a serious problem.

Key words: groundwater, contamination, human health, risk assessment, Jinghui irrigation district

中图分类号: 

  • X523
[1] 赵娟, 李育松, 卞建民, 等. 吉林西部地区高砷地下水砷的阈值分析及风险评价[J]. 吉林大学学报(地球科学版), 2013, 43(1):251-258. Zhao Juan, Li Yusong, Bian Jianmin,et al. Threshold Analysis and Health Risk Assessment of Arsenic in Groundwater in Western Jilin Province[J]. Journal of Jilin University (Earth Science Edition), 2013, 43(1):251-258.
[2] Zhang Y T, Wu J H, Xu B. Human Health Risk Assessmentof Groundwater Nitrogen Pollution in Jinghui Canal Irrigation Area of the Loess Region, Northwest China[J]. Environmental Earth Sciences, 2018, 77(7):273.
[3] 周长松, 邹胜章, 李录娟, 等. 岩溶区典型石灰土Cd形态指示意义及风险评价:以桂林毛村为例[J]. 吉林大学学报(地球科学版), 2016, 46(2):552-562. Zhou Changsong, Zou Shengzhang, Li Lujuan, et al.Implications of Cadmium Forms and Risk Assessment of Calcareous Soil in Karst Area:A Case Study of Maocun in Guilin, China[J]. Journal of Jilin University (Earth Science Edition), 2016, 46(2):552-562.
[4] Li P Y, Li X Y, Meng X Y, et al. Appraising Groundwater Quality and Health Risks from Contamination in a Semiarid Region of Northwest China[J]. Exposure and Health, 2016, 8(3):361-379.
[5] 刘海龙, 马小龙, 袁欣, 等. 基于多元回归分析的铬污染地下水风险评价方法[J]. 吉林大学学报(地球科学版), 2016, 46(6):1823-1829. Liu Hailong, Ma Xiaolong, Yuan Xin, et al.Risk Assessment Method of Chromium(Ⅵ) Polluting Groundwater Based on Multiple Regression Analysis[J]. Journal of Jilin University (Earth Science Edition), 2016, 46(6):1823-1829.
[6] Du S H, Liu Y J, Zhang L J, et al. Assessment of Non-Carcinogenic Health Risks due to Water Contamination in a Loess Distribution Area, Northeastern China[J]. Environmental Earth Sciences, 2017, 76(22):761.
[7] Luu T T, Sthiannopkao S, Kim K W. Arsemic and Other Elements Contamination in Groundwater and a Risk Assessment Study for Resident in the Kandal Province of Cambodia[J]. Environment International, 2009, 35:455-460.
[8] Li P Y, Wu J H, Qian H, et al. Origin and Assessment of Groundwater Pollution and Associated Health Risk:A Case Study in an Industrial Park, Northwest China[J]. Environmental Geochemistry and Health, 2014, 36(4):693-712..
[9] Li P Y, Feng W, Xue C Y, et al. Spatiotemporal Variability of Contaminants in Lake Water and Their Risks to Human Health:A Case Study of the Shahu Lake Tourist Area, Northwest China[J]. Exposure and Health, 2017, 9(3):213-225.
[10] 余葱葱, 赵委托, 高小峰, 等. 电镀厂周边地表水中重金属分布特征及健康风险评价[J]. 环境科学, 2017, 38(3):993-1001. Yu Congcong, Zhao Weituo, Gao Xiaofeng, et al. Distribution Characteristics and Health Risk Assessment of Heavy Metals in Surface Water Around Electroplating Factories[J]. Environmental Science, 2017, 38(3):993-1001.
[11] 易秀, 谷晓静, 侯燕卿, 等. 陕西省泾惠渠灌区土壤重金属环境质量现状及评价[J]. 水土保持通报, 2010, 30(3):153-157. Yi Xiu, Gu Xiaojing, Hou Yanqing, et al. Current Situation and Evaluation of Soil Environmental Quality for Heavy Metals in Jinghuiqu Irrigation District of Shaanxi Province[J]. Bulletin of Soil and Water Conservation, 2010, 30(3):153-157.
[12] 叶遇春. 泾惠渠志[M]. 西安:三秦出版社, 1991. Ye Yuchun. Records of Jinghuiqu[M].Xi'an:Sanqin Press, 1991.
[13] 刘燕, 朱红艳. 泾惠渠灌区水环境劣变特征及地下水调蓄能力分析[J]. 农业工程学报, 2011, 27(6):19-24. Liu Yan, Zhu Hongyan. Characteristicsof Inferior Variation of Water Environment and Regulating Capacity of Groundwater Reservoir in Jinghui Canal Irrigation District of China[J]. Transactions of the CSAE, 2011, 27(6):19-24.
[14] 水质样品的保存和管理技术规定HJ 493-2009[S]. 北京:中国环境科学出版社, 2009. Water Quality-Technical Regulation of the Preservation and Handling of Samples HJ493-2009[S]. Beijing:China Environmental Science Press, 2009.
[15] 中国环境监测总站. 环境水质监测质量保证手册[M]. 北京:化学工业出版社, 2003. China National Environmental Monitoring Centre. Environmental Water Quality Monitoring Manual[M]. Beijing:Chemical Industry Press, 2003.
[16] 生活饮用水卫生标准GB5479-2006[S]. 北京:中国标准出版社, 2006. Standards for Drinking Water Quality GB5479-2006[S]. Beijing:Standards Press of China, 2006.
[17] USEPA. Integrated Risk Information System (IRIS)[EB/OL]. (2017-01-19)[2017-06-24]. http://www.epa.gov/iris/.
[18] USEPA. Risk Assessment Guidance for Superfund (RAGS):Part A[EB/OL]. (2017-01-19)[2017-06-24].https://www.epa.gov/risk/risk-assessment-guidance-superfund-rags-part.
[19] 周艳涛, 张楚怡. 陕西人均预期寿命排全国21位[N]. 华商报, 2010-08-10(A4). Zhou Yantao, Zhang Chuyi. Average Life Expectancy of Shaanxi Ranks 21 in China[N]. Chinese Business View, 2010-08-10(A4).
[20] USEPA. Risk Assessment Guidance for Superfund (RAGS):Volume Ⅲ:Part A[EB/OL]. (2017-01-19)[2017-06-24].https://www.epa.gov/risk/risk-assessment-guidance-superfund-rags-volume-iii-part.
[21] USEPA. Risk Assessment Guidance for Superfund (RAGS):Part E[EB/OL]. (2017-01-19)[2017-06-24].https://www.epa.gov/risk/risk-assessment-guidance-superfund-rags-part-e.
[22] 左娇蕾. 我国四城市成年居民饮水现状的研究[D]. 北京:中国疾病预防控制中心, 2011. Zuo Jiaolei. Current Status Water Intake of Adults in Four Cities of China[D]. Beijing:Chinese Center for Disease Control and Prevention, 2011.
[23] 中华人民共和国国家卫生和计划生育委员会. 疾病预防控制局中国居民营养与慢性病状况报告(2015年)[M]. 北京:人民卫生出版社, 2015. National Health and Family Planning Commission of the PRC. Report on the Status of Nutrition and Chronic Diseases Among Chinese Residents in the Bureau of Disease Control and Prevention(2015)[M]. Beijing:People's Medical Publishing House, 2015.
[24] USEPA. Risk Assessment Guidance for Superfund (RAGS):Part B[EB/OL]. (2017-01-19)[2017-06-24]. https://www.epa.gov/risk/risk-assessment-guidance-superfund-rags-part-b.
[25] 王喆, 刘少卿, 陈晓民, 等. 健康风险评价中中国人皮肤暴露面积的估算[J]. 安全与环境学报, 2008, 8(4):152-156. Wang Zhe, Liu Shaoqing, Chen Xiaomin, et al. Estimates of the Exposed Dermal Surface Area of Chinese in View of Human Health Risk Assessment[J]. Journal of Safety and Environment, 2008, 8(4):152-156.
[26] 张会兴, 张征, 宋莹. 地下水污染健康风险评价理论体系研究[J]. 环境保护科学, 2013, 39(3):59-63. Zhang Huixing, Zhang Zheng, Song Ying. Theoretical System Study on Health Risk Assessment of Groundwater Polution[J]. Environmental Protection Science, 2013, 39(3):59-63.
[27] 余彬. 泾惠渠灌区浅层地下水中重金属的健康风险评价[D]. 西安:长安大学, 2010. Yu Bin. Health Risk Assessment of Heavy Metals in Groundwater in Jinghuiqu Irrigation District[D]. Xi'an:Chang'an University, 2010.
[28] 雷凌明,喻大松,陈玉鹏, 等. 陕西泾惠渠灌区土壤重金属空间分布特征及来源[J]. 农业工程学报, 2014, 30(6):88-96. Lei Lingming, Yu Dasong, Chen Yupeng, et al. Spatial Distribution and Sources of Heavy Metals in Soils of Jinghui Irrigated Area of Shaanxi, China[J]. Transactions of the Chinese Society of Agricultural Engineering, 2014, 30(6):88-96.
[29] 徐斌. 基于空间分析建模的地下水环境演化分析系统[D]. 西安:长安大学, 2015. Xu Bin. Groundwater Environment Evolution Analysis System Based on Spatial Analysis and Modeling[D]. Xi'an:Chang'an University, 2015.
[30] 郭华明, 倪萍, 贾永锋, 等. 原生高砷地下水的类型、化学特征及成因[J]. 地学前缘, 2014, 21(4):1-12. Guo Huaming, Ni Ping, Jia Yongfeng, et al. Types, Chemical Characteristics and Genesis of Geogenic High-Arsenic Groundwater in the World[J]. Earth Science Frontiers, 2014, 21(4):1-12.
[31] 高存荣, 冯翠娥, 刘文波, 等. 地壳表层砷的循环与污染地下水模式[J]. 地球学报, 2014, 25(6):741-750. Gao Cunrong, Feng Cuie, Liu Wenbo, et al. Patterns of Arsenic Cycle and Groundwater Arsenic Contamination on the Earth's Surface[J]. Acta Geoscientica Sinica, 2014, 25(6):741-750.
[32] 梁俊, 赵政阳, 刘振中, 等. 陕西渭北苹果园土壤砷含量与分布特征研究[J]. 西北农林科技大学学报(自然科学版), 2008, 26(11):157-161. Liang Jun, Zhao Zhenyang, Liu Zhenzhong, et al. Study on the Distribution and Contents of Arsenic in Apple Orchard Soils of Weibei, Shaanxi[J]. Journal of Northwest A&F University (Natural Science Edition), 2008, 26(11):157-161.
[33] 李玉浸, 王德中, 宁安荣, 等. 陕西地区主要粮食作物中砷、铬元素背景值及其分布[J]. 农业环境科学学报, 1989, 8(3):13-16. Li Yujin, Wang Dezhong, Ning Anrong, et al. Background and Distribution of Arsenic and Chromium Elements in Main Grain Crops in Shaanxi Province[J].Journal of Agro-Environment Science, 1989, 8(3):13-16.
[34] 易秀, 李佩成. 陕西交口灌区地下水防铬砷污染安全埋深的探讨[J]. 农业环境科学学报, 2005, 24(2):333-336. YiXiu, Li Peicheng. Safely Buried Depth for Protection of Groundwater from Pollution of Cr and As at Jiaokou Irrigation Area in Shaanxi Province[J]. Journal of Agro-Environment Science, 2005, 24(2):333-336.
[35] 韩彩波. 泾惠渠灌区地下水中三氮分布特征及其影响因素的研究[D]. 西安:长安大学, 2010. Han Caibo. The Distribution of Three Nitrogen and Origin Analysis in Groundwater in Jinghuiqu Irrigation Area[D]. Xi'an:Chang'an University, 2010.
[36] 叶媛媛. 泾惠渠灌区地下水水质现状调查分析及其演化规律的研究[D]. 西安:长安大学, 2009. Ye Yuanyuan. Study on the Current Situation and Evolution Law of the Groundwater in Jinghuiqu Irrigation District[D]. Xi'an:Chang'an University, 2009.
[37] 朱参胜, 白广禄, 李跃, 等. 2005年陕西省饮用高砷水筛查和砷中毒病情调查[J]. 中国地方病学杂志, 2007, 26(1):55-57. Zhu Cansheng, Bai Guanglu, Li Yue, et al. Arsenic Contents in Drinking Water and Arsenism Status:Report of a Provincial Survey in Shaanxi Province in 2005[J]. Chinese Journal of Endemiology, 2007, 26(1):55-57.
[38] 地方性砷中毒诊断标准WS/T211-2001[S]. 北京:中国标准出版社, 2001. Diagnosisof Endemic Arsenicosis WS/T211-2001[S]. Beijing:Standards Press of China, 2001.
[39] 陕西省地方病防治研究所. 陕西省饮水型砷中毒流行现况[EB/OL]. (2008-05-23)[2017-06-24]. http://www.sxdfs.com/newstyle/pub_newsshow.asp?id=29004569&chid=100218. Shaanxi Provincial Institute for Endemic Disease Control.Prevalence of Arsenic Poisoning in Drinking Water in Shaanxi Province[EB/OL]. (2008-05-23)[2017-06-24].http://www.sxdfs.com/newstyle/pub_newsshow.asp?id=29004569&chid=100218.
[40] 生活饮用水卫生标准GB5479-85[S]. 北京:中国标准出版社, 1985. Standards for Drinking Water Quality GB5479-85[S]. Beijing:Standards Press of China, 1985.
[41] Yoshida T, Yamauchi H, FanSun G. Chronic Health Effects in People Exposed to Arsenic via the Drinking Water:Dose-Response Relationships in Review[J]. Toxicol Appl Pharmacol, 2004, 198(3):243-252.
[42] 刘秀花. 泾惠渠灌区地下水水质演化过程研究[R]. 西安:长安大学, 2016. Liu Xiuhua. Evolution Process of Groundwater Quality in Jinghuiqu Irrigation District[R]. Xi'an:Chang'an University, 2016.
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